1. 浙江工业大学 能源与碳中和科教融合学院,浙江,杭州,310023
2. 杭州市新能源投资发展有限公司,浙江,杭州,310011
3. 杭州市北京航空航天大学国际创新研究院,浙江,杭州,311115
[ "邓凯(1984—),女,湖北天门人,副教授,博士,研究方向为零碳低氮燃烧技术,E-mail:dkai@zjut.edu.cn" ]
网络出版:2025-03-15,
纸质出版:2025
移动端阅览
邓凯,刘镇宇,蔡路茵,陈建林,梁志荣,何艾迪,叶识恒,林文涛. 声场作用下氨氢旋流预混燃烧NOx排放特性研究动力工程学报, 2025, 45(3): 410-419 https://doi.
org/10.19805/j.cnki.jcspe.2025.230767
邓凯,刘镇宇,蔡路茵,陈建林,梁志荣,何艾迪,叶识恒,林文涛. 声场作用下氨氢旋流预混燃烧NOx排放特性研究动力工程学报, 2025, 45(3): 410-419 https://doi. DOI: 10.19805/j.cnki.jcspe.2025.230767.
org/10.19805/j.cnki.jcspe.2025.230767 DOI:
针对声场作用下氨氢旋流预混火焰NO
x
生成特性
基于OH-PLIF图像测试技术
对声频率为180 Hz和压力振幅为200 Pa的火焰结构进行了分析
通过图像处理技术得到火焰结构及表面密度分布
探讨了不同当量比和掺氢比下燃烧和声场脉动耦合作用对NO
x
排放的影响。结果表明:声场作用能在一定程度上抑制氨氢旋流预混火焰NO
x
的生成
其减排效果受到当量比
Φ
和掺氢比
Z
f
的影响;声场对燃烧流场的影响主要作用于火焰周围的空气
形成周期性脉动流
因此声场对低当量比(
Φ
≤0.8)、以空气动量主导的燃烧场下产生的NO
x
有较好的减排作用
对高当量比(
Φ
>0.8)、以燃料化学反应主导的燃烧场下产生的NO
x
影响较小;声场作用下贫燃火焰表面密度增大
平均OH强度降低
这是因为声场强化了火焰燃烧强度
加快了燃烧速率以及与周围流场的传热传质;当掺氢比较低(0.20≤
Z
f
<0.30)时
声场作用使火焰面积缩小
NO
x
减排幅度相对较高;当掺氢比较高(0.30≤
Z
f
≤0.35)时
对火焰面积的压缩效应减弱
NO
x
减排幅度略有降低。
To investigate the NO
x
formation characteristics of ammonia-hydrogen swirl premixed flames under acoustic excitation
hydroxyl radical plannar laser induced fluorescence (OH-PLIF) imaging technology was used to analyze the flame structure at the sound frequency of 180 Hz an
d the pressure amplitude of 200 Pa. Flame structure and surface density distribution were obtained through image processing techniques. The effects of combustion and acoustic field pulsation coupling on NO
x
emissions under different equivalence ratios (
Φ
) and hydrogen blending ratios (
Z
f
) were explored. Results show that the acoustic field can suppress the formation of NO
x
in ammonia-hydrogen swirl premixed flames to some extent
with the reduction effect influenced by
Φ
and
Z
f
. The acoustic field mainly affects the combustion flow field by creating periodic pulsating flows around the flame
thus demonstrating a better NO
x
reduction effect in combustion fields dominated by air momentum at low equivalence ratios (
Φ
≤0.8). In combustion fields dominated by fuel chemical reactions at high equivalence ratios (
Φ
>0.8)
the effect on NO
x
emissions is less significant. Under the influence of the acoustic field
the surface density of lean flames increases
and the average OH intensity decreases
as the acoustic field enhances flame combustion intensity
accelerates the combustion rate
and improves heat and mass transfer with the surrounding flow field. When the hydrogen blending ratio is low (0.20≤
Z
f
<
0.30)
the acoustic field causes the flame area to shrink
leading to a relatively higher NO
x
reduction. When the hydrogen blending ratio is high (0.30≤
Z
f
≤0.35)
the compressive effect on the flame area weakens
and the NO
x
reduction effect is slightly reduced.
TIAN Jie, WANG Lu, XIONG Yong, et al. Enhancing combustion efficiency and reducing nitrogen oxide emissions from ammonia combustion: a comprehensive review[J]. Process Safety and Environmental Protection, 2024, 183: 514-543.
李晨鹏, 李政, 刘培, 等. 应用无碳氨的氨煤混燃机组平准化电力成本计算[J]. 动力工程学报, 2022, 42(11): 1042-1050. LI Chenpeng, LI Zheng, LIU Pei, et al. Levelized cost calculation of electricity in ammonia-coal co-combustion unit using green ammonia[J]. Journal of Chinese Society of Power Engineering, 2022, 42(11): 1042-1050.
吕强, 王儒儒, 李长兴, 等. 燃煤锅炉掺氨燃烧研究进展[J]. 节能技术, 2023, 41(4): 324-331. LYU Qiang, WANG Ruru, LI Changxing, et al. Research progress on co-firing ammonia in coal-fired boiler[J]. Energy Conservation Technology, 2023, 41(4): 324-331.
中国石油化工股份有限公司, 中石化洛阳工程有限公司, 中石化炼化工程(集团)股份有限公司. 一种燃烧氨及氮气回收工业炉工艺及系统: 202211041548.1[P]. 2024-03-08.
LI Jun, HUANG Hongyu, DENG Lisheng, et al. Effect of hydrogen addition on combustion and heat release characteristics of ammonia flame[J]. Energy, 2019, 175: 604-617.
OKAFOR E C, YAMASHITA H, HAYAKAWA A, et al. Flame stability and emissions characteristics of liquid ammonia spray co-fired with methane in a single stage swirl combustor[J]. Fuel, 2021, 287: 119433.
FRANCO M C, ROCHA R C, COSTA M, et al. Characteristics of NH3/H2/air flames in a combustor fired by a swirl and bluff-body stabilized burner[J]. Proceedings of the Combustion Institute, 2021, 38(4): 5129-5138.
DA ROCHA R C, COSTA M, BAI Xuesong. Chemical kinetic modelling of ammonia/hydrogen/air ignition, premixed flame propagation and NO emission[J]. Fuel, 2019, 246: 24-33.
SOMARATHNE K D K A, HAYAKAWA A, KOBAYASHI H. Numerical investigation on the combustion characteristics of turbulent premixed ammonia/air flames stabilized by a swirl burner[J]. Journal of Fluid Science and Technology, 2016, 11(4): JFST0026.
KURATA O, IKI N, INOUE T, et al. Development of a wide range-operable, rich-lean low-NOx combustor for NH3 fuel gas-turbine power generation[J]. Proceedings of the Combustion Institute, 2019, 37(4): 4587-4595.
KHATEEB A A, GUIBERTI T F, ZHU Xuren, et al. Stability limits and NO emissions of technically-premixed ammonia-hydrogen-nitrogen-air swirl flames[J]. International Journal of Hydrogen Energy, 2020, 45(41): 22008-22018.
ROCHA R C, COSTA M, BAI Xuesong. Combustion and emission characteristics of ammonia under conditions relevant to modern gas turbines[J]. Combustion Science and Technology, 2021, 193(14): 2514-2533.
钟英杰, 邓凯, 李华, 等. 声场作用下甲烷部分预混火焰NOx生成特性实验研究[J]. 工程热物理学报, 2011, 32(9): 1609-1612. ZHONG Yingjie, DENG Kai, LI Hua, et al. Experimental study of NOx emission in partially premixed flame under acoustic forcing[J]. Journal of Engineering Thermophysics, 2011, 32(9): 1609-1612.
邓凯. 脉动燃烧下甲烷部分预混火焰NOx生成机理和排放规律研究[D]. 杭州: 浙江工业大学, 2010.
金晶, 许林云, 张爱琪, 等. 不同尾管数量的全浸入式脉动燃烧器传热特性试验[J]. 林业工程学报, 2023, 8(1): 157-164. JIN Jing, XU Linyun, ZHANG Aiqi, et al. Experimental study on heat transfer characteristics of fully immersed pulsation combustors with different numbers of tailpipes[J]. Journal of Forestry Engineering, 2023, 8(1): 157-164.
徐艳英, 翟明, 董芃, 等. 弯尾管Helmholtz型无阀自激脉动燃烧器NOx排放特性[J]. 热力发电, 2015, 44(2): 18-23. XU Yanying, ZHAI Ming, DONG Peng, et al. NOx emission characteristics of a Helmholtz valveless self-excited pulse combustor with bend tailpipe[J]. Thermal Power Generation, 2015, 44(2): 18-23.
SIVASEGARAM S, TSAI R F, WHITELAW J H. Control of oscillations and NOx concentrations in ducted premixed flames by spray injection of water[R]. New York, USA:American Society of Mechanical Engineers, 1995.
AU-YEUNG H W, GARNER C P, HANBY V I. An experimental study of the effects of combustion frequency and pressure amplitude on the NO emissions from pulse combustors[J]. Journal of the Institute of Energy, 1998, 71(489): 204-208.
邓凯, 钟英杰, 李华, 等. 甲烷自激励脉动燃烧NOx排放特性的试验研究[J]. 动力工程学报, 2010, 30(7): 528-535. DENG Kai, ZHONG Yingjie, LI Hua, et al. Experimental study on NOx emission from methane self-excited pulsating combustion[J]. Journal of Chinese Society of Power Engineering, 2010, 30(7): 528-535.
邓凯, 沈忠良, 王明晓, 等. 当量比对脉动燃烧NOx生成机理的影响[J]. 燃烧科学与技术, 2014, 20(5): 428-432. DENG Kai, SHEN Zhongliang, WANG Mingxiao, et al. NOx formation mechanism of pulse combustion under different equivalence ratios[J]. Journal of Combustion Science and Technology, 2014, 20(5): 428-432.
JOO S, YOON J, KIM J, et al. NOx emissions characteristics of the partially premixed combustion of H2/CO/CH4 syngas using artificial neural networks[J]. Applied Thermal Engineering, 2015, 80: 436-444.
袁逸人, 孙培锋, 葛冰, 等. 贫预混预蒸发燃烧室的火焰结构及污染物排放[J]. 燃烧科学与技术, 2018, 24(5): 451-457. YUAN Yiren, SUN Peifeng, GE Bing, et al. Flame structure and pollution emissions in a lean premixed prevaporized combustor[J]. Journal of Combustion Science and Technology, 2018, 24(5): 451-457.
吕志超, 洪洋, 赵国江. 掺混H2对CH4-空气对冲扩散火焰温度和NOx生成影响的数值研究[J]. 可再生能源, 2022, 40(9): 1144-1148. LV ZhiChao, HONG Yang, ZHAO Guojiang. Numerical study on the influence of H2 addition on flame temperature and NOx production of CH4-air opposed-flow diffusion flame[J]. Renewable Energy Resources, 2022, 40(9): 1144-1148.
ZHANG Meng, AN Zhenhua, WANG Liang, et al. The regulation effect of methane and hydrogen on the emission characteristics of ammonia/air combustion in a model combustor[J]. International Journal of Hydrogen Energy, 2021, 46(40): 21013-21025.
DENG Kai, XUE Chenyang, LIU Zhenyu, et al. Analysis of combustion instability of methane-air premixed swirling flame based on OH-PLIF measurements[J]. ACS Omega, 2023, 8(9): 8664-8674.
0
浏览量
2
下载量
0
CSCD
关联资源
相关文章
相关作者
相关机构
京公网安备11010802024621