1. 大连海事大学物理系
2. 大连海事大学轮机工程学院
网络出版:2018-03-30,
纸质出版:2018
移动端阅览
张芝涛, 高颖, 李日红, 等. 近大气压DBD氧等离子体化学反应效能[J]. 高电压技术, 2018,44(3):849-855.
ZHANG Zhitao, GAO Ying, LI Rihong, et al. Efficiency of ROS Generation Generated by Dielectric Barrier Discharge Near Atmosphere[J]. 2018, 44(3): 849-855.
大气压介质阻挡放电(dielectric barrier discharge
DBD)氧等离子体发生模块是高级氧化水处理技术中的重要组件
其等离子体化学反应效能直接影响实际应用中的处理效率。通过测量大气压DBD氧等离子体发生模块在不同工作气压下的放电参数及活性氧粒子产生浓度
探究了工作气压对氧等离子体化学反应效能的影响。结果显示
工作气压的降低使得氧等离子体反应模块的等效电容与放电气隙的折合场强度增强
导致在施加不同功率时
模块表现出不同的放电特性与等离子体化学反应效能。当电源功率低于150 W时
活性氧产生效能随工作气压降低而增大
当电源功率在175
2
50 W范围内时
活性氧产生效能随工作气压的降低先增大后减小
当电源功率高于275 W时
活性氧产生效能随工作气压降低而减小。工作气压降低时活性氧最高浓度减小
当工作气压为60、70、80、90和100 k Pa时
活性氧最高质量浓度分别为127.3、143.1、149.7、152.1和157.7 g/m
3
。为使活性氧产生效能最大
需根据实际状况不同
采用不同的电源功率
使活性氧发生模块处于最佳工作状态。
Reactive oxygen species(ROS) generation module based on DBD is an important part in advanced oxidation technology. ROS generation efficiency affects the production efficiency in practical application. We researched the effect of working pressure on generation module
and analyzed discharge parameters and ROS concentration. The results show that the module equivalent capacitance will increase and the electric field intensity will reduce with the depression of pressure. Therefore
there are different discharge characteristics for different input power in the module
during which the ROS generation efficiency is different. If the input power is below 150 W
ROS generation efficiency will increase with the reduction of pressure. If the input power ranges from 175 W to 250 W
the efficiency will increase to maximum with the reduction of pressure
and then it decreases. If the input power is higher than 275 W
ROS concentration will reduce with the reduction of the pressure. If the pressure reduces
the maximum of ROS concentration will reduce too. When the pressure are 60
70
80
90 and 100 k Pa
the corresponding ROS concentration maximums are 127.3
143.1
149.7
152.1
and 157.7 g/m3
respectively. To ensure that the ROS generation module keeps the best work condition
a suitable power needs to be used according to the actual situations.
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