YI Shanting, LIU Feng, FANG Zhi. Discharge Characteristics of Ar/NH3/H2O Plasma Jet Under Atmospheric Pressure[J]. 2019, 45(6): 1936-1944.DOI:
大气压Ar/NH3/H2O等离子体射流放电特性
摘要
为提高等离子体射流在材料表面处理、环境保护及消毒灭菌等领域中的应用效果
通过在大气压Ar等离子体射流中添加适量NH
3
/H
2
O气体
增强等离子体射流活性。利用发射光谱诊断和发光图像拍摄
研究Ar/NH
3
/H
2
O等离子体射流NH、OH、O等强氧化性粒子发射光谱强度及射流长度随外加电压和添加气体含量的变化规律
测量相应条件下电压电流波形和Lissajous图形
并对实验结果做机理分析与讨论。研究结果表明
Ar/NH
3
/H
2
O等离子体射流主要产生Ar、N
2
、NH、OH和O等粒子。随外加电压增大
NH、OH和O等粒子谱线强度、射流长度、放电功率和传输电荷均随之增大。当NH
3
在Ar/NH
3
气体体系中体积分数达到0.012 5%时
NH自由基发射光谱强度达到最大。在此条件下添加H
2
O
发现当H
2
O体积分数达到0.25%时
OH和O粒子谱线强度达到最大
比Ar/NH
3
放电时OH和O粒子谱线强度分别增加了104.4%和55.8%
而NH粒子谱线强度则下降了18.7%
此时等离子体射流中氧化性粒子(NH、OH和O)总发射光谱强度达到最大
更有利于在材料亲水改性和消毒灭菌等方面应用。
Abstract
To enhance the treatment effects of the atmospheric pressure plasma jet(APPJ) in the fields of material surface treatment
environmental protection
and disinfection sterilization
etc.
NH
3
/H
2
O were added to the Ar APPJ to improve the activity of the APPJ. The optical emission spectral intensities of NH
OH and O and the length of the plasma plume were investigated at various applied voltages and NH
3
/H
2
O ratios by optical emission spectra diagnosis and light-emission images
observation. The voltage-current waveforms and Lissajous figures were also recorded correspondingly. Results showed that the main species produced by APPJ in Ar/NH
3
/H
2
O included Ar
N
2
NH
OH
and O. As the applied voltage increased
the emission spectral intensities of NH
OH and O
the length of the plasma plume
discharge power and transported charges all increased. When the added NH
3
reached 0.012 5% in the Ar/NH
3
mixed gas
the emission spectral intensity of NH reached the maximum.
When H
2
O was added under this condition
it was found that the emission spectral intensities of OH and O reached the maximum values when the water vapor content was 0.25% and the emission spectral intensities of OH and O increased by 104.4% and 55.8% as compared with those of APPJ in Ar/NH
3
while the emission spectral intensity of NH decreased by 18.7%. The overall emission spectral intensities of the oxidizing particles(NH
OH and O) in Ar APPJ reached the maximum
and it should be more favorable for applications in materials hydrophilic modification and disinfection sterilization