Polypropylene (PP)-based recyclable materials have attracted tremendous interest for HVDC cable insulation applications due to their superior electrical properties

e.g.

high thermal stability and superior recyclability. Compared with crosslinked polyethylene (XLPE)

PP-based materials exhibit the advantages of not only higher working temperatures but also facile and efficient cable manufacturing with reduced costs

which are highly desirable in HVDC cable manufacturing. Considering their promising advantages

PP-based materials have received significant attention from both academia and industry in the field of HVDC cable insulation. In order to adopt PP as a cable insulation material

the mechanical flexibility of PP should be improved. However

regulations of the mechanical properties inevitably influences the electrical properties of PP. So extensive research has been conducted on the regulation of the mechanical and electrical properties of PP. This review summarizes the research progress on recyclable PP-based materials for HVDC cable insulation applications. Particular attention is placed on the electrical property regulations and material structure-property relationships. The challenges that remain to be addressed and the opportunities for future studies on PP-based recyclable HVDC cable insulation materials are also presented.