Recent Advances of CO<sub>2</sub> Conversion Based on DBD

Honglei DING; Detong GUO; Weiguo PAN; Chenggang DING; Shiyi GUO; Yanxing PAN; Qi ZHOU; Wei DU

doi:10.12096/j.2096-4528.pgt.19009

English Version Reader LoginJournal Login

您当前的位置：

首页 >

文章列表页 >

Recent Advances of CO₂ Conversion Based on DBD

Power Generation and Environmental Protection | 更新时间：2025-06-06

- Recent Advances of CO₂ Conversion Based on DBD
- Power Generation Technology Vol. 40, Issue 5, Pages: 481-487(2019)
- 作者机构：
  
  1.上海电力学院能源与机械工程学院, 上海市杨浦区 200090
  2.上海电气电站环保工程有限公司, 上海市静安区 201600
  3.上海发电环保工程技术研究中心, 上海市杨浦区 200090
- 作者简介：
- 基金信息：
- DOI：10.12096/j.2096-4528.pgt.19009
  CLC：
- Received：16 January 2019，
  
  Published：2019-10
- 稿件说明：
移动端阅览
Honglei DING, Detong GUO, Weiguo PAN, et al. Recent Advances of CO₂ Conversion Based on DBD[J]. Power Generation Technology, 2019, 40(5): 481-487.
DOI：

Honglei DING, Detong GUO, Weiguo PAN, et al. Recent Advances of CO₂ Conversion Based on DBD[J]. Power Generation Technology, 2019, 40(5): 481-487. DOI： 10.12096/j.2096-4528.pgt.19009.

摘要

为了更高效地进行CO

的转化利用，许多学者开展了多种CO

转化方法的研究。介电阻挡放电（dielectric barrier discharge，DBD）能在低温常压的环境下还原CO

，是CO

转化利用的重要方法之一。为了设计出更好的DBD反应器、更佳的反应条件和催化剂，总结了近年来DBD转化CO

的相关研究。通过分析不同研究中过程参数、稀释性气体和催化剂等因素对CO

转化量和能量效率的影响，发现催化剂能大幅度提高DBD转化CO

的反应效率，并介绍了DBD中一些常用的催化剂。最后简要分析了此类研究的可能发展趋势。

Abstract

In order to convert CO

more efficiently

many scholars have carried out research on various CO

conversion methods. Dielectric barrier discharge (DBD) is one of the important methods of CO

conversion and utilization

it can reduce CO

under the condition of low temperature and normal pressure. In order to design a better DBD reactor

reaction conditions and catalysts

this paper summarized the researches on CO

conversion based on DBD in recent years. The effects of process parameters

diluting gases and catalysts on CO

conversion and energy efficiency in different studies were analyzed. It was found that the catalyst can greatly improve the efficiency of CO

conversion by DBD

and introduced some commonly used catalysts in DBD. Finally

the possible development trend of CO

conversion by DBD was briefly analyzed.

关键词

Keywords

references

Rogelj J, Den E M, Höhne N, et al.Paris agreement climate proposals need a boost to keep warming well below 2℃[J].Nature, 2016, 534(7609):631-639.

毛健雄.燃煤电站CO 2 减排技术的探讨[J ] .分布式能源, 2017, 2(1):35-43.

Zheng Y, Wen Q, Li F, et al.Energy related CO 2 conversionand utilization:Advanced materials/nanomaterials, reaction mechanisms and technologies[J ] .Nano Energy, 2017, 4:512-539.

孔飞, 王思韬, 马翊洋, 等.等离子体改性对环氧树脂材料表面电荷动态特性的影响[J].广东电力, 2018, 31(8):161-166.

Bogaerts A, Kozak T, van Laer K, et al.Plasma-based conversion of CO 2 :current status and future challenges[J ] .Faraday Discussions, 2015, 183:217-232.

Sergey Y S, Hwaung L, Song H K, et al.The decomposition of CO 2 in glow discharge[J ] .Journal of Chemical Engineering, 2002, 19(4):564-566.

Horvath, G, Skalny J D, Mason N J.FTIR study of decomposition of carbon dioxide in DC corona discharges[J].Journal of Physics D:Applied Physics, 2008, 41(22):207-225

Abramski K M, Colley A D, Baker H J, et al.Power scaling of large area transverse radio frequency discharge CO 2 lasers[J ] .Applied Physics Letters, 1989, 54(19):1833-1835.

Wang W Z, Mei D H, Tu X, et al.Gliding arc plasma for CO 2 conversion:better insights by a combined experimental and modelling approach[J ] .Chemical Engineering Journal, 2017, 330:11-25.

Chen G X, Godfroid T, Britun N, et al.Plasma-catalytic conversion of CO 2 and CO 2 /H 2 O in a surface-wave sustained microwave discharge[J ] .Applied Catalysis B:Environmental, 2017, 214:114-125..

Sadat H, Dubus N, Tatibouet J M.Temperature runaway in a pulsed dielectric barrier discharge reactor[J].Applied Thermal Engineering, 2012, 37:324-328.

Snoeckx R, Bogaerts A.Plasma technology:a novel solution for CO 2 conversion[J ] .Chemical Society Reviews, 2017, 46(19):5805-5863.

Mei D H, Tu X.Conversion of CO 2 in a cylindrical dielectric barrier discharge reactor:effects of plasma processing parameters and reactor design[J ] .Journal of CO 2 Utilization, 2017, 19:68-78..

Ray D, Saha R, Subrahmanyam C.DBD plasma assisted CO 2 decomposition:influence of diluent gases[J ] .Catalysis, 2017, 7(9):244-250.

Wang L, Yi Y H, Guo H C, et al.Atmospheric pressure and room temperature synthesis of methanol through plasma-catalytic hydrogenation of CO 2 [J ] .ACS Catalysis, 2017, 8(1):90-100.

Nunnally T, Gutsol K, Rabinovich A, et al.Dissociation of CO 2 in a low current gliding arc plasmatron[J ] .Journal of Physics D:Applied Physics, 2011, 44(27):274-290.

Fridman A.Plasma Chemistry[M].New York:Cambridge University Press, 2008.

Chen P, Shen J, Ran T C, et al.Investigation of operating parameters on CO 2 splitting by dielectric barrier discharge plasma[J ] .Plasma Science and Technology, 2017, 19(12):123-128.

Snoeckx R, Heijkers S, Wesenbeeck Van K, et al.CO 2 conversion in a dielectric barrier discharge plasma:N 2 in the mix as a helping hand or problematic impurity[J ] .Energy & Environmental Science, 2016, 9(3):999-1011..

Xu S J, Whitehead J C, Martin P A.CO 2 conversion in a non-thermal, barium titanate packed bed plasma reactor:the effect of dilution by Ar and N 2 [J ] .Chemical Engineering Journa l, 2017, 327:764-773..

Zeng Y X, Tu X.Plasma-catalytic hydrogenation of CO 2 for the cogeneration of CO and CH 4 in a dielectric barrier discharge reactor:effect of argon addition[J ] .Journal of Physics D:Applied Physics, 2017, 50(18):184-190..

Mei D H, Zhu X B, He Y L, et al.Plasma-assisted conversion of CO 2 in a dielectric barrier discharge reactor:understanding the effect of packing materials[J ] .Plasma Sources Science & Technology, 2015, 24(1):11-15.

Ray D, Subrahmanyam C.CO 2 decomposition in a packed DBD plasma reactor:influence of packing materials[J ] .RSC Advances, 2016, 6(96):93997-93999.

Tu X, Whitehead J C.Plasma-catalytic dry reforming of methane in an atmospheric dielectric barrier discharge:understanding the synergistic effect at low temperature[J].Applied Catalysis B:Environmental, 2012, 125:439-448.

Kattel S, Yan B H, Chen J G, et al.CO 2 hydrogenation on Pt, Pt/SiO 2 and Pt/TiO 2 :importance of synergy between Pt and oxide support[J ] .Journal of Catalysis, 2016, 343:115-126..

Li K, Yin C, Zheng Y, et al.DFT Study on the methane synthesis from syngas on a Cerium-Doped Ni (111) surface[J].Journal of Physical Chemistry C, 2016, 120(40):23030-23043.

Choe S J, Kang H J, Kim S J, et al.Adsorbed carbon formation and carbon hydrogenation for CO 2 methanation on the Ni (111) surface:ASED-MO study[J ] .Bulletin of the Korean Chemical Society, 2005, 26(11):1682-1688.

Zeng Y X, Zhu X B, Mei D H, et al.Plasma-catalytic dry reforming of methane over γ-Al 2 O 3 supported metal catalysts[J ] .Catalysis Today, 2015, 256:80-87..

黄秋实.Ni基催化剂与等离子体协同作用下的CO 2 甲烷化[D ] .大连: 大连理工大学, 2017.

杨志强.低温等离子体协同催化CO 2 甲烷化反应研究[D ] .大连: 大连理工大学, 2014.

Zeng Y X, Tu X.Plasma-catalytic CO 2 hydrogenation at low temperatures[J ] .IEEE Transactions on Plasma Science, 2016, 44(4):405-411.

Falbo L, Martinelli M, Visconti C G, et al. Kinetics of CO 2 methanation on a Ru-based catalyst at process conditions relevant for power-to-gas applications[J ] .Applied Catalysis B:Environmental, 2018, 225:354-363.

Garbarino G, Bellotti D, Finocchio E, et al.Meth-anation of carbon dioxide on Ru/Al 2 O 3 :catalytic activity and infrared study[J ] .Catalysis Today, 2016, 277:21-28..

Mebrahtu C, Abate S, Perathoner S, et al.CO 2 methanation over Ni catalysts based on ternary and quaternary mixed oxide:a comparison and analysis of the structure-activity relationships[J ] .Catalysis Today, 2018, 304:181-189.

Lim Y G, McGregor J, Sederman A J, et al.Kinetic studies of CO 2 methanation over a Ni/γ-Al 2 O 3 catalyst using a batch reactor[J ] .Chemical Engineering Science, 2016, 141:28-45..

Ocampo F, Louis B, Roger A C, et al.Methanation of carbon dioxide over nickel-based Ce 0.72 Zr 0.28 O 2 mixed oxide catalysts prepared by sol-gel method[J ] .Applied Catalysis A:General, 2009, 369:90-96..

Le A T, Kim S M, Lee S H, et al.CO and CO 2 methanation over supported Ni catalysts[J ] Catalysi s Today, 2017, 293/294:89-96.

Jwa E, Lee S B, Lee H W, et al.Plasma-assisted catalytic methanation of CO and CO 2 over Ni-zeolite catalysts[J ] .Fuel Processing Technology, 2013, 108(6):89-93.

Mei D H, Zhu X B, Wu C F, et al.Plasma-photocatalytic conversion of CO 2 at low temperatures:understanding the synergistic effect of plasma-catalysis[J ] .Applied Catalysis B:Environmental, 2016, 182:525-532.

Ahmad W, Younis M N, Shawabkeh R, et al.Synthesis of lanthanide series (La, Ce, Pr, Eu & Gd) promoted Ni/γ-Al 2 O 3 catalysts for methanation of CO 2 at low temperature under atmospheric pressure[J ] .Catalysis Communications, 2017, 100:121-126..

张丽.等离子体和助剂改性镍基催化剂二氧化碳甲烷化研究[D].天津: 天津大学, 2015.

Mihet M, Lazar M D.Methanation of CO 2 on Ni/-Al 2 O 3 :influence of Pt, Pd or Rh promotion[J ] .Catalysis Today, 2016, 304:286-290..

Liu Q, Gu F N, Gao J J, et al.Ni/Al 2 O 3 -ZrO 2 catalyst for CO 2 methanation:the role of γ-(Al, Zr) 2 O 3 formation[J ] .Catalysis Today, 2018, 306:294-299..

Lim J Y, McGregor G, Sederman A J, et al.The role of the Boudouard and water-gas shift reactions in the methanation of CO or CO 2 over Ni/γ-Al 2 O 3 catalyst[J ] .Chemical Engineering Science, 2016, 152:754-766..

Mebrahtu C, Abate S, Chen S M, et al.Enhanced catalytic activity of Fe-promoted Ni over γ-Al 2 O 3 nanosheets for CO 2 methanation[J ] .Energy Technology, 2017, 6(6):1196-1207..

Benrabbah R, Cavaniol C, Liu H, et al.Plasma DBD activated ceria-zirconia-promoted Ni-catalysts for plasma catalytic CO 2 hydrogenation at low temperature[J ] .Catalysis Communications, 2017, 89:73-76.

Nizio M, Albarazi A, Cavadias S, et al.Hybrid plasma-catalytic methanation of CO 2 at low temperature over ceria zirconia supported Ni catalysts[J ] .International Journal of Hydrogen Energy, 2016, 41(27):11584-11592.

聂望欣, 邹秀晶, 汪学广, 等.介孔γ-Al 2 O 3 负载的高分散Ni-Ce-Zr氧化物的制备及其二氧化碳甲烷化研究(英文)[J ] .物理化学学报, 2016, 32(11):2803-2810..

Bie C D, Dijk J V, Bogaerts A.CO 2 hydrogenation in a dielectric barrier discharge plasma revealed[J ] .Journal of Physical Chemistry C, 2016, 120(44):1123-1129.

Studt F, Behrens M, Kunkes E L, et al.The mechanism of CO and CO 2 hydrogenation to methanol over Cu-based catalysts[J ] .Chem Cat Chem, 2015, 44(27):182-190.

Eliasson B, Kogelschatz U, Xue B, et al.Hydroge-nation of carbon dioxide to methanol with a discharge-activated catalyst[J].Industrial&Engineering Chemistry Research, 1998, 37(8):3350-3357.

Bradford M C J, Vannice M A.CO 2 reforming of CH 4 [J ] .Catalysis Reviews, 2007, 41(1):1-42..

Bie C D, Dijk J V, Bogaerts A.The dominant pathways for the conversion of methane into oxygenates and syngas in an atmospheric pressure dielectric barrier discharge[J].Journal of Physical Chemistry C, 2015, 119(39):22331-22350.

Zeng Y X, Wang L, Wu C F, et al.Low temperature reforming of biogas over K-, Mg-and Ce-promoted Ni/Al 2 O 3 catalysts for the production of hydrogen rich syngas:understanding the plasma-catalytic synergy[J ] .Applied Catalysis B:Environmental, 2018, 224:469-478..

Amin M H, Putla S, Hamid S B, et al.Understanding the role of lanthanide promoters on the structure:activity of nanosized Ni/-Al 2 O 3 catalysts in carbon dioxide reforming of methane[J ] .Applied Catalysis A:General, 2015, 492:160-168..

Pham M H, Goujard V, Tatibouët J M, et al.Activation of methane and carbon dioxide in dielectric-barrier discharge-plasma reactor to produce hydrocarbons-influence of La 2 O 3 /γ-Al 2 O 3 catalyst[J ] .Catalysis Today, 2011, 171:67-71..

Ray D, Reddy P M K, Subrahmanyam C.Ni-Mn/γ-Al 2 O 3 assisted plasma dry reforming of methane[J ] .Catalysis Today, 2017, 309:212-218..

Views

下载量

CSCD

Alert me when the article has been cited

提交

Tools

Publicity Resources

Structure Design and Optimization of Helium Cooling Tube for Nuclear Fusion Poloidal Coil

Research and Application of Numerical Simulation for Selective Catalytic Reduction Denitration of 9F Gas Turbine

Research Progress of Hydrogen Production by Methanol Reforming for Fuel Cell Power Generation

Related Author

ZOU Chunlong

DU Shuangsong

JIANG Feng

LU Kun

WEI Jing

SHEN Guang

Peter Readman

ZHANG Hongyi

Related Institution

Institute of Plasma Physics, Chinese Academy of Sciences

Hefei CAS Ion Medical and Technical Device Co., LTD.

Fusion for Energy

Tianjin Branch Co., Ltd., China Huadian Group Co., Ltd., Binhai District

Huadian Electric Power Research Institute Co., Ltd.

AI问答

⁰

Recent Advances of CO2 Conversion Based on DBD

DOI：10.12096/j.2096-4528.pgt.19009

摘要

Abstract

关键词

Keywords

references

Recent Advances of CO₂ Conversion Based on DBD