Low temperature plasma technology can be used to treat the refractory biodegradable organic compound. There are many strong oxidizing active species (such as H2O2
·OH
O3) in the plasma channel when voltage discharge is high. A needle-plate reactor was used to investigate the generation of H2O2 in the pulsed discharge system. The effects of different experimental conditions on H2O2 generation
such as discharge voltage
gas flow rate
electrode gap and pH value
were studied. Experimental results show that as discharge voltage increases
the concentration of H2O2 in water increases; when the gas flow rate is 1.6 L/min
the concentration of H2O2 is the highest in water. The electric intensity increases as the electrodes gap decreases
and thus the东concentration of H2O2 increases.
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references
Sun B, Sato M, Clements J S.Optical study of active species produced by a pulsed streamer corona discharge in water [J].Journal of Electrostatics, 1997, 39: 189-202.
Yang B, Zhou M H, Lei L C.Synergistic effects of liquid and gas phase discharges using pulsed high voltage for dyes degradation in the presence of oxygen [J].Chemosphere, 2005, 60: 405-411.
Li J, Zhou Z G, Wang H J, et al.Research on decoloration of dye wastewater by combination of pulsed discharge plasma and TiO2 nanoparticles [J].Desalination, 2007, 212: 123-128.
Zhang Y Z, Deng S H, Sun B Y, et al.Preparation of TiO2-loaded activated carbon fiber hybrids and application in a pulsed discharge reactor for decomposition of methyl orange [J].Journal of Colloid and Interface Science, 2010, 347: 260-266.
Magureanu M, Piroi D, Mandache N B, et al.Degradation of pharmaceutical compound pentoxifylline in water by non-thermal plasma treatment [J].Water Research, 2010, 44: 3445-3453.
Satoh K, Macgregor S J, Anderson J G, et al.Pulsed-Plasma disinfection of water containing Escherichia coli [J].Japanese Journal of Applied Physics, 2007, 46(3): 1137-1141.
Miao H, Yun G.The sterilization of Escherichia coli by dielectric-barrier discharge plasma at atmospheric pressure [J].Applied Surface Science, 2011, 257(16): 7065-7070.
Lukes P, Appleton A T, Locke B R.Hydrogen peroxide and ozone formation in hybrid gas-liquid electrical discharge reactors [J].IEEE Transactions on Industry Applications, 2004, 40(1): 60-67.