严亚伦, 胡艺嵩, 冯英杰. 不同燃料包壳在高温高压水中的表面腐蚀产物沉积行为研究[J]. 核科学与工程, 2022, 42(6): 1260-1267.
引用本文: 严亚伦, 胡艺嵩, 冯英杰. 不同燃料包壳在高温高压水中的表面腐蚀产物沉积行为研究[J]. 核科学与工程, 2022, 42(6): 1260-1267.
YAN Yalun, HU Yisong, FENG Yingjie. Study on the Deposition Behavior of Surface Corrosion Products of Different Fuel Cladding in High Temperature and High Pressurized Water[J]. Chinese Journal of Nuclear Science and Engineering, 2022, 42(6): 1260-1267.
Citation: YAN Yalun, HU Yisong, FENG Yingjie. Study on the Deposition Behavior of Surface Corrosion Products of Different Fuel Cladding in High Temperature and High Pressurized Water[J]. Chinese Journal of Nuclear Science and Engineering, 2022, 42(6): 1260-1267.

不同燃料包壳在高温高压水中的表面腐蚀产物沉积行为研究

Study on the Deposition Behavior of Surface Corrosion Products of Different Fuel Cladding in High Temperature and High Pressurized Water

  • 摘要: 压水堆一回路材料腐蚀产物在燃料包壳表面沉积会形成燃料污垢。燃料污垢可能引起垢致轴向功率偏移(CrudInducedPowerShift,CIPS)和包壳垢致局部腐蚀(CrudInducedLocalized Corrosion,CILC)。腐蚀产物的沉积与燃料包壳表面特性相关,例如表面粗糙度等。Cr涂层锆合金是一种典型的事故容错燃料(Accident Tolerant Fuel,ATF)包壳。Cr涂层可能改变锆合金包壳表面的特性,进而改变腐蚀产物在燃料包壳表面的沉积行为。本论文通过试验研究了锆合金包壳和Cr涂层锆合金包壳在高温高压水中的表面腐蚀产物沉积行为。试验后采用扫面电子显微镜(Scanning Electric Microscope,SEM)对污垢的表面和截面的形貌和成分进行分析。结果表明,Cr涂层锆合金包壳表面污垢成分含有Cr元素;Cr涂层锆合金包壳表面污垢无明显烟囱状结构,锆合金包壳表面烟囱状结构明显,且烟囱面密度约为127个/mm2;Cr涂层锆合金包壳表面污垢平均厚度比锆合金包壳表面的污垢厚度减小约6μm。

     

    Abstract: The deposition of corrosion products of primary circuit materials of PWR on the surface of fuel cladding will form fuel crud. The fuel crud may cause crud induced power shift (CIPS) and crud induced local corrosion(CILC). The deposition of corrosion products is related to the surface characteristics of fuel cladding, such as surface roughness. The Cr-coated-Zr cladding is a typical kind of accident tolerant fuel(ATF) cladding. The Cr coating may change the characteristics of the Zr cladding surface, and then change the deposition behavior of corrosion products on the fuel cladding surface. In this paper, the deposition behavior of corrosion products on the surface of the Zr cladding and Cr-coated-Zr cladding in high temperature and high pressurized water was studied by experiment. After the experiment, the morphology and composition of the crud surface and section were analyzed by scanning electron microscope(SEM). The results showed that the crud on the surface of the Cr-coated-Zr cladding contained Cr; there was no obvious chimney-like structure on the surface of the Cr-coated-Zr cladding, but the chimney-like structure on the surface of the Zr cladding was obvious, and the chimney surface density was about 127/mm2; the average crud thickness on the surface of the Cr-coated-Zr cladding was about 6 μm less than that on the surface of the Zr cladding.

     

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